Structural changes of polystyrene particles in subcritical and supercritical water revealed by in situ small-angle neutron scattering

Shibata, Motoki*; Nakanishi, Yohei*; Abe, Jun*; Arima, Hiroshi*; Iwase, Hiroki*; Shibayama, Mitsuhiro*; Motokawa, Ryuhei; Kumada, Takayuki; Takata, Shinichi; Yamamoto, Katsuhiro*; et al.

Polymer Journal, 55(11), p.1165 - 1170, 2023/11

https://doi.org/10.1038/s41428-023-00817-1

Random media criticality analysis methods in Monte Carlo solver Solomon

Ueki, Taro

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 9 Pages, 2023/10

A Monte Carlo Solver Solomon has been under development as an object-oriented code written in the C++14 standards. It consists of regular capabilities of criticality safety analysis and a special capability of random media criticality. In the latter capability, Solomon is equipped with a class for the random media modeled by the incomplete randomized Weierstrass function (IRWF). By this modeling, the uncertainty of random media criticality can be evaluated by executing criticality calculations over many IRWF-replicas. However, it is impossible to know beforehand how many IRWF-replicas should be computed. To deal with this issue, a bounded amplification (BA) technique has been newly equipped in Solomon. Applying BA to IRWF, it is possible to reduce the number of IRWF-replicas by more than 95% in terms of the upper limit estimation of neutron effective multiplication factor. Solomon is also equipped with a voxel-overlay (VO). This functionality is shown to be valuable for evaluating the resonance self-shielding effect.

The Nuclear criticality accident in Japan, Revisited

Okuno, Hiroshi; Suyama, Kenya

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10

The criticality accident that resulted in the evacuation of residents occurred on September 30, 1999, at JCO's nuclear fuel fabrication plant in Ibaraki prefecture, Japan. This paper presents the outline, technical issues and background of the accident and the situations that followed. The review of this accident was one of the hot issues in the last ICNC2003 organized in Tokai-mura. At the this turn of ICNC in Japan, we would like to revisit the accident to reaffirm and share the idea that the response and preparedness should be strengthened to protect people and the environment from nuclear disasters. The accident occurred in a factory of JCO during the informal and unusual process of preparing a uranium nitrate solution of medium-enriched (18.8 weight% U) uranium from UO using the precipitation tank of 45 cm in diameter, which exceeded the critical diameter (ca. 23 cm) of an infinite cylinder with a full thick water reflector. A 2.2-cm-thick water "jacket" surrounded and enclosed the tank, and the jacket was connected to the cooling tower beside the factory. The jacket not only functioned as the neutron reflector but also prevented the evaporation of the solution, and then the criticality continued for about 20 hours. Because JCO's plant had not anticipated the criticality accident, the response to the accident was confusing. During the accident, the JAERI and JNC, both the predecessors of the Japan Atomic Energy Agency (JAEA), acted to terminate the criticality and reduce the residents' exposure to radiation. After the accident, the JAERI and the National Institute of Radiological Sciences provided the telephone consultation at the village office of Tokai-mura. The JNC did the same things at the prefectural building of Ibaraki to advise the residents. The presentation may include issues of applying the Slide rule, identifying a nuclear criticality accident to occur, and responding to the emergency.

Planning of the debris-simulated critical experiments on the new STACY

Gunji, Satoshi; Araki, Shohei; Arakaki, Yu; Izawa, Kazuhiko; Suyama, Kenya

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 9 Pages, 2023/10

JAEA has been modifying a critical assembly called STACY from a solution system to a light-water moderated heterogeneous system to validate computation results of criticality characteristics of fuel debris generated in the accident at TEPCO's Fukushima Daiichi Nuclear Power Station. To experimentally simulate the composition and characteristics of fuel debris, we will prepare several grid plates which make particular neutron moderation conditions and a number of rod-shaped concrete and stainless-steel materials. Experiments to evaluate fuel debris's criticality characteristics are scheduled using these devices and materials. This series of STACY experiments are planned to measure the reactivity of fuel debris-simulated samples, measure the critical mass of core configurations containing structural materials such as concrete and stainless steels, and the change in critical mass when their arrangement becomes non-uniform. Furthermore, two divided cores experiments are scheduled that statically simulate fuel debris falling, and also scheduled that subcriticality measurement experiments with partially different neutron moderation conditions. The experimental plans have been considered taking into account some experimental constraints. This paper shows the schedule of these experiments, as well as the computation results of the optimized core configurations and expected results for each experiment.

Debris-simulated core analysis under fuel procurement constraints in new STACY experiments

Araki, Shohei; Gunji, Satoshi; Arakaki, Yu; Yoshikawa, Tomoki; Murakami, Takahiko; Kobayashi, Fuyumi; Izawa, Kazuhiko; Suyama, Kenya

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10

New experiments simulating fuel debris in the new criticality assembly, STACY, are designed to contribute to the validation of criticality calculations for criticality control of the fuel debris in the Fukushima Daiichi Nuclear Power Plant accident. In the new STACY experiment, a two-region core consisting of a driver region and a test region was investigated in order to configure a debris-simulated core with under-moderation condition (lattice pitch 1.27-cm) having the constraint of available fuel rod number. The test region with a 1.27-cm lattice pitch is surrounded by the driver region, in which fuel rods are arranged in a checkerboard pattern on a 1.27-cm lattice plate, with a 1.80-cm lattice pitch. Neutron spectra and sensitivity were calculated by using MCNP6 and ENDF/B-VII. The core which has a 1717 test region with 373 fuel rods is the largest two-region core under the constraint. It was found that the core which has a 1717 test region can simulate the neutron spectra of under-moderation condition in a 1313 region inside the test region with the root-mean square percentage error of less than 5%. It was also confirmed that the sensitivity of Si and Ca (n,) reactions when the concrete simulant, was loaded could be simulated.

Development of experimental core configurations to clarify k variations by nonuniform core configurations

Gunji, Satoshi; Araki, Shohei; Suyama, Kenya

Nuclear Science and Engineering, 197(8), p.2017 - 2029, 2023/08

https://doi.org/10.1080/00295639.2022.2164151

The fuel debris generated by the accident at the Tokyo Electric Power Company's Fukushima Daiichi Nuclear Power Plant is expected to have not only heterogeneous but also nonuniform compositions. Similarly, damaged fuel assemblies remaining in the reactor vessels also have nonuniform configurations due to some missing fuel rods. This non-uniformity may cause changing neutron multiplication factors. The effect of non-uniformity on the neutron multiplication factor is clarified by computations, and the possibility of experimentally validating the computations used for criticality management is being investigated. For this purpose, in this study the criticality effects of several core configurations of a new critical assembly, STACY, of the Japan Atomic Energy Agency with nonuniform arrangements of uranium oxide fuel rods, concrete rods, and stainless-steel rods were studied to confirm benchmarking potential. The difference in these arrangements changed the neutron multiplication factor by more than 1 $. We confirmed that changes in local neutron moderation conditions and the clustering of specific components caused this effect. In addition, the feasibility of benchmark experimental cores with nonuniform arrangements is evaluated. If benchmarking of such experiments could be realized, it would help to validate calculation codes and to develop criticality management methods by machine learning.

Preliminary analysis of randomized configuration patterns in modified STACY core

Shiba, Shigeki*; Iwahashi, Daiki*; Okawa, Tsuyoshi*; Gunji, Satoshi; Izawa, Kazuhiko; Suyama, Kenya

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 9 Pages, 2023/05

The Nuclear Regulation Authority (NRA) has tackled the experimental approach for determining the criticality of pseudo-fuel debris plausibly simulating actual fuel debris since 2014, collaborating with the Japan Atomic Energy Agency. To elucidate the characteristics of the pseudo-fuel debris, the Japan Atomic Energy Agency modified the STACY (STAtic experiment Critical facilitY) to conduct critical experiments simulating fuel debris. Thus, we proposed three types of modified STACY core configurations. In critical experiments in the modified STACY core, it is important to judge whether the proposed modified STACY core configurations are representative of molten core-concrete interaction debris or not. In this study, we built pseudo-fuel debris models considering a volume ratio of pseudo-fuel debris to moderation (V/V) and calculated uncertainty-based similarity values (C) between the modified STACY core configurations and pseudo-fuel debris models using Tools for Sensitivity and Uncertainty Analysis Methodology Implementation-Indices and Parameters (TSUNAMI-IP) in SCALE 6.2. Consequently, the modified STACY core configuration loading structure rods we proposed completely resulted in high similarity to the pseudo-fuel debris models through V/V values. The main contributions to C values were U , U , and Fe (n,), except for the pseudo-fuel debris model, including extremely high concrete components.

Direct measurement of the evolution of magnetism and superconductivity toward the quantum critical point

Higemoto, Wataru; Yokoyama, Makoto*; Ito, Takashi; Suzuki, Taiga*; Raymond, S.*; Yanase, Yoichi*

Proceedings of the National Academy of Sciences of the United States of America, 119(49), p.e2209549119_1 - e2209549119_6, 2022/11

https://doi.org/10.1073/pnas.2209549119

no abstracts in English

Completion of JENDL-5 and prospects for its application to numerical analysis, 4; Integral test of JENDL-5; Benchmark analysis in fast reactor system

Yokoyama, Kenji; Taninaka, Hiroshi

Kaku Deta Nyusu (Internet), (132), p.25 - 33, 2022/06

http://www.aesj.or.jp/~ndd/ndnews/pdf132/No132-04.pdf

This article explains the results of integral test of JENDL-5 by benchmark analysis in fast reactor system, which were presented in a special session of the 2022 Spring Annual Meeting of the Atomic Energy Society of Japan (AESJ). The latest version of Japanese evaluated nuclear data library, JENDL-5, was released in December 2021. In order to confirm the applicability of JENDL-5 to the fast reactor system, we conducted a set of benchmark analysis using the integral experiment data included in the fast reactor nuclear design database which is being developed by JAEA. With respect to major nuclear characteristics in the standard fast reactor system, it was confirmed that the ratios of analysis result and experimental result (C/E values) based on JENDL-5 were almost the same as those of JENDL-4.0. In the special session, the results of sensitivity analysis were reported. Since the results have been described in the proceedings of the AESJ meeting, we add the results of the versions under development of JENDL-5 and discuss their relationship with the reported results of sensitivity analysis.

Evaluation of critical experimental core configurations to simulate non-uniform fuel debris

Gunji, Satoshi; Araki, Shohei; Suyama, Kenya; Izawa, Kazuhiko

Proceedings of International Conference on Physics of Reactors 2022 (PHYSOR 2022) (Internet), 10 Pages, 2022/05

The fuel debris is expected to have not only heterogeneous but also non-uniform compositions. Therefore, the calculation method used in their criticality management is required to be validated experimentally. In this study, several core configurations of a new critical assembly "STACY" of JAEA with non-uniform arrangements of uranium oxide fuel rods, concrete rods and stainless steel rods, which are components of the fuel debris, were studied. In each case, the median value of 100 sample patterns was larger than the mean effective multiplication factor. It was also confirmed that there are differences in the effective multiplication factor of more than one dollar by the pattern changing, and that the neutron spectra can change significantly by changing the local neutron moderation conditions. In particular, the effective multiplication factor became smaller when over-moderated regions with large water-to-fuel ratios were formed in the core configurations due to increases in thermal neutron absorption. Such criticality experiments with non-uniform arrangements of multiple compositions will be useful to evaluate the validity of the calculation code.